Does smoke from burning different things change the sky to different colors?
Research question: Do smoke particles from different fuels scatter sunlight differently enough to tint the sky in different shades?
The records show that smoke's scattering behavior depends more on burn conditions than on fuel type alone, because single-scattering albedo cannot be predicted from fuel type alone 1. Some fuel-linked differences do appear: Indonesian peat smoke scatters strongly at 532 and 660 nm but absorbs more blue light at 405 nm 2, and single-scattering albedo at 405 nm varied from 0.37 to 0.95 across fuel types 4. Combustion efficiency was estimated to explain about 60% of the variability in smoke single-scattering albedo, with the remaining 40% possibly due to fuel type 18. None of these facts measure sky color or tint directly, so they only partly answer whether these differences would visibly tint the sky; the newest dated fact in the set is from 2020 11.
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"SSA and AAE cannot be directly predicted based on fuel type because they depend strongly on burn conditions."Parameterization of single-scattering albedo (SSA) and absorption Ångström exponent (AAE) with EC / OC for aerosol emissions from biomass burning (2016)
"Notably, these parameterizations are effective for emissions from Indonesian peat, which have very little black carbon but significant brown carbon (SSA = 0.990 ± 0.001 at 532 and 660 nm, SSA = 0.937 ± 0.011 at 405 nm)."Parameterization of single-scattering albedo (SSA) and absorption Ångström exponent (AAE) with EC / OC for aerosol emissions from biomass burning (2016)
"Utilizing spectral irradiance data, the model retrieved values of ω0decreased with increasing wavelength, with the change of ω0as a function of wavelength differing on different days."Measurements of irradiance attenuation and estimation of aerosol single scattering albedo for biomass burning aerosols in Amazonia (1998)
"Single scattering albedo values at 405 nm ranging from 0.37 to 0.95 were measured for different fuel types"Strong spectral variation of biomass smoke light absorption and single scattering albedo observed with a novel dual‐wavelength photoacoustic instrument (2008)
"single‐scattering albedo averages 0.87 ±0.08 at 670 nm"Single‐scattering albedo of smoke retrieved from the sky radiance and solar transmittance measured from ground (1998)
"Values of ω0, at approximately 550 nm, estimated from this technique using broadband 400–700 nm irradiance measurements, ranged from approximately 0.82 to 0.94 for the dates and times of these SCAR‐B measurements."Measurements of irradiance attenuation and estimation of aerosol single scattering albedo for biomass burning aerosols in Amazonia (1998)
"For biomass smoke, Ångström exponents as high as 3.5 were found in association with smoke having single scattering albedo near unity."Strong spectral variation of biomass smoke light absorption and single scattering albedo observed with a novel dual‐wavelength photoacoustic instrument (2008)
"Typically between 0.7 and 0.95” this statement is not always true for BBsmoke. Therearelotsoflaboratoryandambientstudieswhichshowsahugerange of SSA from BB emissions"Review of "Inter-comparison of biomass burning aerosol optical properties from in-situ and remote-sensing instruments in ORACLES-2016" (2019)
"The spectral dependence of the single‐scattering albedo has both tendencies: decreasing and increasing with wavelength."Single‐scattering albedo of smoke retrieved from the sky radiance and solar transmittance measured from ground (1998)
"An absorption Ångström exponent near unity is commonly observed for motor vehicle emission‐generated black carbon aerosol."Strong spectral variation of biomass smoke light absorption and single scattering albedo observed with a novel dual‐wavelength photoacoustic instrument (2008)
"The simulations show that both MAE and MSE can exhibit strong and diverse changes during BB aerosol evolution mostly due to significant changes in the aerosol particle size distribution."Effects of physical and chemical nonlinearities on evolution of optical properties of biomass burning aerosol (2020)
"Across all five regions, wildfire-derived BrC exhibits substantial absorption not only in the near-ultraviolet and short-wavelength visible range (~400 nm), but also in the mid- to long-visible wavelengths (500–700 nm)."Strong global radiative effects from wildfire dark brown carbon - Nature
"These aerosols exhibit substantial absorption across the visible spectrum, with mass absorption efficiencies (MAE OC ) between 0.5 and 1.5 m 2 g −1 at ~500 nm."Strong global radiative effects from wildfire dark brown carbon - Nature
"In several wildfire events, BrC absorption at visible wavelengths equals or even surpasses that of BC, highlighting BrC as a substantial absorber."Strong global radiative effects from wildfire dark brown carbon - Nature
"Notably, they are considerably lower than those typically reported for weakly absorbing BrC, which generally range from 4 to 11 in literature"Strong global radiative effects from wildfire dark brown carbon - Nature
"Results show that ω varies strongly with fire‐integrated modified combustion efficiency (MCEFI)—higher MCEFI results in lower ω values and greater spectral dependence of ω."Aerosol single scattering albedo dependence on biomass combustion efficiency: Laboratory and field studies (2013)
"These properties are related to fuel type, fire intensity, combustion efficiency, and particle composition."Physical and optical properties of young smoke from individual biomass fires in Brazil (1998)
"The parameterization suggests that MCEFI explains 60% of the variability in ω, while the 40% unexplained variability could be accounted for by other parameters such as fuel type."Aerosol single scattering albedo dependence on biomass combustion efficiency: Laboratory and field studies (2013)
"The wavelength dependence of ω0varied significantly over the region, with greater decreases for increasing wavelength at smoke‐dominated sites than for sites influenced by a significant coarse mode aerosol component."Variability of biomass burning aerosol optical characteristics in southern Africa during the SAFARI 2000 dry season campaign and a comparison of single scattering albedo estimates from radiometric measurements (2003)
"The optical properties of smoke from individual biomass fires in Brazil differ significantly from those of smoke from biomass burning in North America."Physical and optical properties of young smoke from individual biomass fires in Brazil (1998)
"other aerosols including fossil fuel burning, industrial, and aeolian coarse mode types also contributed to the aerosol mixture in other regions (South Africa and Mozambique)"Variability of biomass burning aerosol optical characteristics in southern Africa during the SAFARI 2000 dry season campaign and a comparison of single scattering albedo estimates from radiometric measurements (2003)
"In particular, the total light‐scattering coefficient for smoke particles in Brazil is, on average, 15% less than for smoke particles in North America."Physical and optical properties of young smoke from individual biomass fires in Brazil (1998)
"as a result of both methods retrieving the imaginary index of refraction (∼0.030–0.035 on one day) with very little wavelength dependence."Variability of biomass burning aerosol optical characteristics in southern Africa during the SAFARI 2000 dry season campaign and a comparison of single scattering albedo estimates from radiometric measurements (2003)
"Also, the average values of the single‐scattering albedos of smoke particles in Brazil are 0.05 to 0.1 less than those in North America."Physical and optical properties of young smoke from individual biomass fires in Brazil (1998)
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